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Vanadium redox flow batteries (VRFBs) operate effectively over the temperature range of 10 °C to 40 °C. However, their performance is significantly compromised at low operating temperatures, which may happen in cold climatic conditions. . The main mass transfer processes of the ions in a vanadium redox flow battery and the temperature dependence of corresponding mass transfer properties of the ions were estimated by investigating the influences of temperature on the electrolyte properties and the single cell performance. A. . Using a mixed solution of sulfuric acid and hydrochloric acid as a supporting solution, the operating temperature of the all-vanadium Redox-flow battery was extended to the range of -5~50 °C at a vanadium concentration of 3. This is due to the complex chemistry of the pentavalent vanadium, which tends to co dense irrever-sibly to vanadium pentoxide at around 40 °C. The loss of performance can be attributed to reduced kinetics. . To address this challenge, a novel aqueous ionic-liquid based electrolyte comprising 1-butyl-3-methylimidazolium chloride (BmimCl) and vanadium chloride (VCl 3) was synthesized to enhance the solubility of the vanadium salt and aid in improving the efficiency. The synthesized novel electrolyte. .
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