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This study analyzes an alternative membrane-free (membraneless) flow battery technology that relies on immiscible electrolytes, which spontaneously separate into two distinct liquid phases, eliminating the need for an ion-selective membrane or any other kind of physical separator. . Redox flow batteries (RFBs) are particularly suitable due to their efficiency and unique ability to decouple energy and power density. However, their widespread adoption is hindered by the high costs of ion-selective membranes and vanadium-based electrolytes currently used in commercial vanadium. . A flow battery, or redox flow battery (after reduction–oxidation), is a type of electrochemical cell where chemical energy is provided by two chemical components dissolved in liquids that are pumped through the system on separate sides of a membrane. [1][2] Ion transfer inside the cell (accompanied. . This technology strategy assessment on flow batteries, released as part of the Long-Duration Storage Shot, contains the findings from the Storage Innovations (SI) 2030 strategic initiative. The objective of SI 2030 is to develop specific and quantifiable research, development, and deployment (RD&D). . Membrane-free redox flow batteries (RFBs) are promising energy-storage technologies that present an innovative solution to address the critical need for sustainable and efficient energy systems. Unlike traditional lithium-ion or lead-acid batteries, flow batteries offer longer life spans, scalability, and the ability to discharge for extended durations. These. . This chapter explores the role of ionic liquids (ILs) in enhancing the performance of RFBs, focusing on their potential to overcome conventional limitations. We provide a comprehensive overview of various RFB types, including All-Vanadium, Zinc-Bromine, Iron-Chromium, Aqueous Organic, Metal-Air. .
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